The article referred to at the jqueryvsmootools website puts it quite nicely:
If jQuery makes the DOM your playground, MooTools aims to make JavaScript your playground
So, coupled with the answer here "If it aint broke, don't fix it", I'd say address your needs and not public opinion.
Given that your site is already in Mootools, you need to assess whether jQuery offers anything you need which MooTools doesn't offer; and whether the bother of converting is less than the bother of writing the extension.
It seems that jQuery has the ability to quickly allow you to play with the DOM, but all the extra fancy stuff and other areas of work (like Dates) requires a plugin.
This helped me to answer my own question too!
There are some areas where they don't overlap, which is a pity. GUIs are easy to put together in jQuery, with lovely widgets and animations. MooTools, I find, either have sets with too few features, or are too heavy for general web use.