Let's pretend it's for word frequency counts in a web crawler. Is relational the way to go (I'm imagining a simple two-column table) or is there a NoSQL option better suited to this task?
When I say better, I mean more conceptually suited to the task. I'm not really concerned with scalability, just simplicity and an obvious conceptual mapping to the task at hand. In the way that, for me at least, CouchDB maps much more sensibly to a blog than MySQL does.