[...] bulletproof [...]
Impossible.
Limiting by account will help - IP addresses are far to dynamic and easily changeable to be remotely "secure". You then of course have to limit account creation, again, difficult..
Stackoverflow does it quite nicely (there was blog-entry about this recently, "New Question / Answer Rate Limits") - basically have accounts where you have to actively participate for a while before you can vote. Then you are rate-limited (by account) until you've participated for a bit longer. Then the limits are removed, so you don't annoy more active (more trusted) users.
If you just want to prevent causal, "accidental" voting, limit by cookie, and possibly also by IP (bearing in mind more than one user can be behind a single IP).. If you want to try and prevent abuse, require accounts which you can't just click "signup" for (or rather, one you cannot write a "click signup 2000 times"-script for), although this isn't always possible (or practical)